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Among several advantageous, additive manufacturing facilitates rapid prototyping and the realization of objects that cannot be made with traditional manufacturing methods. Recently, additive manufacturing of magnetic structures is being investigated including the inkjet [1], Fused Filament Modelling (FFM) [2], and UV Assisted Direct Write methods [3]. Soft or hard magnetic particles are included in polymer binder to realize objects interesting for magnetic shielding, magnetic flux guiding, or for their permanent magnetic properties. Magnetic characterization of 3D printed samples with a Vibrating Sample Magnetometer (VSM) however is not straightforward, particularly when larger samples are characterized that have a non-zero infill percentage. Determination of the saturation magnetization is difficult because of the lack of calibration standards for such inhomogeneous samples. Therefore, we modeled the sensitivity of a biaxial VSM for different 3D printed samples produced by FFM. The magnetic potential of a distributed coil with finite dimensions was approximated from the first 3 Legendre polynomial terms and used to determine the point dipole sensitivity of a MicroSense VSM employing a Mallinson pickup coil set using an approach similar as described in [4]. The obtained point sensitivity function was used to calculate the sample signal of various 3D printed samples with different infill orientations and infill percentages using Mathematica. The calculations show that the measured signal is strongly affected by the infill percentage and orientation. For 2D shaped samples (1x1x0.05 cm3) with low infill percentages, the signal differs by up to a factor 2 depending on the sample orientation. The calculated signal of cubed samples (1x1x1 cm3) can vary as much as 30% with infill percentage. A Mathematica spreadsheet was developed that allows one to calculate the signal produced by any specific 3D printed sample in a biaxial VSM that employs a Mallinson coil set configuration. This work was supported in part by NSF through an DMR-MRI Grant under Award 1726970.References: [1] M.P. Paranthaman, C.S. Shafer, M. Elliot, JOM 68 (2017) 1978. [2] C. Huber, C. Abert, F. Bruckner, et al., App. Phys. Lett. 109 (2016) 162401. [3] Alan Shen, Xiaoguang Peng, Callum P. Bailey et al., Mater. and Des.183 (2019) 108133. [4] Co-Cr layers for perpendicular magnetic recording, J.P.C. Bernard, C.P.G. Schrauwen, PhD. Thesis University of Twente, ISBN 90-9003454-4.

MMM 2020

Effect of Field Orientation and Infill Percentage on the VSM calibration factor of FFM 3D printed samples

The 65th Annual Conference on Magnetism and Magnetic Materials (MMM 2020) was held in a virtual form. The COVID-19 pandemic, with its associated uncertainty about international travel and the ability to gather in large groups, meant that the Steering Committee decided to cancel the face-to-face meeting that had been planned in Palm Beach, Florida November 2-6, 2020.

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technical paper

Magnons and phonons are two elementary excitations associated with spin waves and lattice vibrations in solids. In the presence of magneto-elastic interactions, the coupling of the spin and lattice degrees of freedom leads to the formation of a new type of hybridized excitation, i.e., magnon-polarons. Manifested as anomalies in the spin Seebeck effect (SSE) in a ferrimagnet YIG, magnon-polarons have profound consequences in modifying the magnon and phonon dispersion relations and affecting spin transport properties in ferrimagnetic insulators. In antiferromagnetic insulators, the magnon spectrum is distinctly different due to the existence of two equivalent, antiferromagnetically coupled spin sub-lattices. Here we report an observation of antiferromagnetic magnon-polarons in Cr2O3, a prototypical uniaxial antiferromagnet, featured as anomalies in the SSE signals of Cr2O3/heavy metal heterostructures. Despite the relatively high magnon energy in the absence of an external magnetic field, near the spin-flop transition of ~ 6 T, the left-handed magnon spectrum shifts downward to intersect those of acoustic phonons (both longitudinal and transverse) to cause hybridization. We have measured the temperature dependence of the SSE magnon-polaron anomalies in Cr2O3 and revealed the strength of the magneto-elastic coupling. Our study indicates that the hybridized excitations can be employed to manipulate spin transport in antiferromagnetic systems. This work was supported as part of the SHINES, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Basic Energy Sciences under Award No. SC0012670.

Observation of magnon-polarons in a uniaxial antiferromagnetic insulator Cr2O3

Searching for the efficient manipulation of antiferromagnets for spintronic applications, we study the properties of the magnetic domain walls with due account of magnetoleastic effects. We show that magnetoelastic coupling induces anisotropy of the domain wall orientation which affects the shape and distribution of the domain walls in a sample. In case of non-1800 domains such anisotropy favours formation of the plane walls oriented along or perpendicular the hard magnetic axis. We study the pinning effects caused by magnetoelasticity and calculate the frequency of the localized oscillations and depinning field for an easy-plane antiferromagnet. We further consider dynamics of excitations of magnetoelastic domain wall and show that such a wall effectively scatters the long-wave magnons. The scattering and pinning effects are more pronounced in case of non-1800 domains, due to the strain-induced anisotropy inside domains. However, 1800 domain wall can also scatter the magnons due to the magnetoelastic strains inside the wall.To illustrate possible applications of our results we discuss the magnon propagation in multidomain hematite and NiO.

Domain Walls in Antiferromagnets with Strong Magnetoelastic Coupling

The prospect of using antiferromagnets as the main component in logic devices has gained a lot of interest. Antiferromagnets offer many benefits over their ferromagnetic counterparts: terahertz dynamics, no device cross-talk, and robustness to external fields. However, the latter property makes them difficult to control and has hindered their potential for use in spintronics devices. Recently, electrical switching of antiferromagnets has been demonstrated using current-induced spin-orbit torques due to bulk crystal symmetry1,2,3, or spin-transfer torque from a neighbouring heavy metal layer4,5,6. Changes to the magnetic state are typically detected electrically in the transverse anisotropic magnetoresistance, which depends on the angle between the antiferromagnetic Néel vector and the direction of the probe current. This method is effective for measuring the average Néel vector orientation, but provides limited information on the microscopic magnetic texture. We study current-induced modification of the antiferromagnetic domain structure in CuMnAs microdevices using X-ray photoemission electron microscopy (XPEEM). Magnetic contrast is obtained due to X-ray magnetic linear dichroism, i.e. dependence on the angle between the magnetic moments and the incident X-ray polarisation. Our results show a current-induced motion of both 90° and 180° domain walls, in a direction which depends on the polarity of the current pulse (Fig.1). This is an important step towards the development of low power antiferromagnetic domain wall memory devices. Furthermore, 180° domain walls are topologically protected making them particularly good candidates for non-volatile applications.References: 1 P. Wadley et al. Electrical switching of an antiferromagnet. Science, 2016. 2 J. Godinho et al. Electrically induced and detected Néel vector reversal in a collinear antiferromagnet. Nature Communications, 2018. 3 S. Yu. Bodnar et al. Writing and reading antiferromagnetic Mn2Au by Néel spin-orbit torques and large anisotropic magnetoresistance. Nature Communications, 2018. 4 X. Z. Chen et al. Antidamping-torque-induced switching in biaxial antiferromagnetic insulators. Physical Review Letters, 2018. 5 M. Dunz et al. Spin-orbit torque induced electrical switching of antiferromagnetic MnN. Physical Review Research, 2020. 6 P. Zhang et al. Quantitative study on current-induced effect in an antiferromagnet Insulator/Pt bilayer film. Physical Review Letters, 2019.

Electrical control of antiferromagnetic domain walls

With high frequency spin dynamics, stability in the presence of external magnetic fields, and a lack of stray fields, antiferromagnetic materials are positioned to become key in future low power spintronic devices [1]. Here, we study the spin transport in high quality thin films of hematite (α-Fe2O3) (< 500 nm) of different orientations. Through measurements of the spin Hall magnetoresistance in hematite/Pt bilayers, the magnetic anisotropies of the thin films can be extracted, and the critical temperature of the Morin transition from the easy plane to the easy axis antiferromagnetic phase is electrically observed [2]. We find that the strain introduced by the growth process tilts the antiferromagnetic anisotropy axis, leading to complex signals across the full temperature range investigated [3]. Whilst a key part of antiferromagnetic spintronics is to encode and read information in the Néel vector, the efficient transfer of information is crucial for integration of antiferromagnets into devices. Recently, we demonstrated that a diffusive magnon current can be carried over micrometres in antiferromagnetic single crystals, but such crystals are not suitable for spintronic devices [4]. While mechanisms for the long-distance propagation of pure spin currents carried by the antiferromagnetic order [5, 6] have been developed for thin film antiferromagnets, experimentally the long distance transport of angular momentum by magnons has previoulsy not been achieved [7]. Making use of hematite thin films, a robust magnon current can propagate with intrinsic diffusion lengths of hundreds of nanometres [8]. The efficiency of the transport mechanisms can be tuned by the domain structure, the growth orientation, and the relative orientations of the magnetic field and magnetic anisotropies. Finally, we achieve room temperature magnon transport, where the films present an easy plane anisotropy, by dilute substitution of the ferric ions in order to alters the magnetic anisotropy axes of the thin films.References: [1] T. Jungwirth, J. Sinova, A. Manchon et al., Nat. Phys. 14, 200-203 (2018) [2] R. Lebrun, A. Ross, O. Gomonay et al., Comm. Physics 2 50 (2019) [3] A. Ross, R. Lebrun, C. Ulloa et al., arXiv:2001.03117 (2020) [4] R. Lebrun, A. Ross, S. Bender et al., Nature 561, 222-225 (2018) [5] S. Takei, B. Halperin, A. Yacoby et al., Phys. Rev. B, 90, 94408 (2014) [6] S. Bender, H. Skarsvåg, A. Brataas et al., Phys. Rev. Lett. 19, 056804 (2017) [7] H. Wang, C. Du, P. C. Hammel et al., Phys. Rev. B 91, 220410 (2015) [8] A. Ross, R. Lebrun, O. Gomonay et al., Nano Letters 20 1, 306-313 (2020)

Efficient Magnon Transport in Insulating Antiferromagnets Governed by Domain Structures and Doping

Voltage-controlled spintronic devices utilizing the spin degree of freedom are desirable for future applications, and may allow energy-efficient information processing. A pure spin current can be created by thermal excitations in magnetic systems via the spin Seebeck effect (SSE). However, controlling such spin currents, by purely electrical means, has been a fundamental challenge. Here, we investigate voltage control of the SSE in an antiferromagnetic insulator. We demonstrate that the SSE response generated in this material can be effectively controlled by applying a bias voltage, owing to the sensitivity of the SSE to the orientation of the magnetic sublattices as well as the existence of magnetoelectric couplings in the present system. Our experimental results on the voltage-controlled switching of magnetic sublattices are explained using a model based on the magnetoelectric effect. Acknowledgments: all work at Argonne was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The use of facilities at the Center for Nanoscale Materials, an Office of Science user facility, was supported by the US Department of Energy, Basic Energy Sciences under Contract No. DE-AC02-06CH11357.

Voltage control of magnon spin currents in an antiferromagnetic insulator

Ferrimagnetic thulium iron garnet (Tm3Fe5O12 or TIG) grown on GGG substrate is known to have perpendicular magnetic anisotropy and magnetic compensation [1,2]. We investigated magnetization configuration of bismuth and gallium substituted Tm3Fe5O12 films by anomalous Hall effect (AHE) induced in a proximately coupled Pt film, and by x-ray magnetic circular dichroism (XMCD) between 10-200 K. In the TIG/Pt heterostructure, anomalous Hall hysteresis changes sign first at 135 K and then at around 60 K. Besides, above 135K, three hysteresis loops are formed under small (less than 1T) field sweep and in a wide temperature range (135-200K). XMCD measurement confirms 135 K as the compensation temperature, and shows that there is no magnetic moment flip around 60 K. Hence the sign change of AHE at 60 K is attributed to competition between spin Hall effect and magnetic proximity effect contributions. XMCD result also demonstrates that above compensation point, both Fe and Tm sublattice moment flips three times under field sweep at a fixed temperature, while their magnitude remains unchanged. This behavior is not likely from canted spin phase in ferrimagnet [3] since spin canting typically requires a field much larger than 1 T. The reason for this field-induced sublattice moment reorientation is unclear yet.References: [1] C. Tang et al., Phys. Rev. B 94, 140403 (2016). [2] Q. Shao et al., Phys. Rev. B 99, 104401 (2019). [3] J. Bernasconi and D. Kuse, Phys. Rev. B 3, 811 (1971).

Magnetization configuration of Bi and Ga substituted Tm3Fe5O12 probed by proximate anomalous Hall effect and x-ray magnetic circular dichroism

Magneto-dielectric materials have been recently attracting great attention owing to their significant advantages for miniaturization of antennas.1,2 Precise measurement of permeability and permittivity over a wide frequency range is crucial to develop and evaluate advanced magneto-dielectric materials.3,4 The Nicolson-Ross-Weir (NRW) method is widely used to extract electromagnetic constitutive parameters from measured scattering parameters.5 One of the drawbacks of this method is requiring direct measurement of the actual sample position in the measurement fixture, which leads to uncertainty in the measured permeability and permittivity. In this work, we improve the standard NRW method by removing the need for prior knowledge of sample position. For any isotropic material, the sample position in the measurement fixture can be precisely determined by matching the phasor angles of the reflection coefficients at the sample surfaces. The phasor matching algorithm is verified by two kinds of magneto-dielectric materials, ferrite ceramics and ferrite/polymer composites, measured in two sets of test fixtures of different geometries. The uncertainty is independent of the actual sample position along the measurement cell as shown in Fig. 1. The measured permeability and permittivity spectra of the ferrite sample are plotted in Fig. 2, showing quite small and stable standard deviations at lower frequencies. The experimental results indicate that the improved NRW method reduces the errors in calculated permeability and permittivity by one order of magnitude compared to those obtained by the conventional NRW method. Therefore, the proposed position-independent NRW method is a precise, efficient and statistically robust technique to characterize the electromagnetic properties of magneto-dielectric materials over a wide frequency range.References: 1R. C. Hansen and M. Burke, Microw. Opt. Technol. Lett., Vol. 26, no. 2, p. 75 (2000). 2K. Buell, H. Mosallaei, and K. Sarabandi, IEEE Trans. Microw. Theory Tech., Vol. 54, p. 135 (2006). 3Q. Li, Y. Chen, C. Yu et al., J. Am. Ceram. Soc., Vol. 105, (2020). 4Q. Li, Y. Chen, and V. G. Harris, J. Appl. Phys., Vol. 125, p. 185107 (2019). 5J. R. Baker-Jarvis, Nat. Inst. Stands. Tech. Tech. Note 1341, (1990).

A Position-Independent Approach to Accurate Measurement of Broadband Electromagnetic Constitutive Parameters of Magneto-Dielectric Materials

Magnetic characterization is an undeniable scheme for the identification of magnetic and mechanical properties of materials [1] [2]. More pertinent is the unavoidable urge for localized magnetic monitoring schemes in line with the current growing industrial expectations [3] [4]. Herein, the adequacy and consistency of the magnetic needle probe (MNP) method over the conventional search coil method were concealed by the instrumentation prerequisite coupled to very weak levels of the sensor signals and the limited theoretical investigation on the method, generally considered quite blurry. The first hindrance taken care of by technological upgrades, studies on the basis of the electromagnetic theory from eddy-current distribution in magnetic materials has advanced the interpretation of the MNP method for local magnetic measurements [5] [6]. The objectives of this paper are twofold; it presents an electromagnetic modelling of the MNP method in a rectangular bar from a micro-magnetic perspective and exploits the model to derive the magnetic anhysteretic behaviour of the ferromagnetic materials. In the first objective, the advance theoretical background of the MNP method is modelled for anti-parallel domain structure using Finite Difference (FD) approach and compared to the analytical approach in [5]. Then, the model is used to simulate the reversible stochastic motion of domain walls for a hysteresis free magnetic material. The dependence of the anhysteretic model on the domain width (d) and the ratio of domain width to the thickness (d/c) of a Fe-3%Si sheet tells of the sensitivity of the magnetic microstructure on the magnetic signature. Noticeable hysteresis losses were however observed at smaller domain width translating to a state of high magneto-crystallographic anisotropy where closure domain effects add the resultant magnetization in the magnetic material. A complete account of the domain constituency is envisaged for future studies.References: [1] Y. A. Tene, P. Tsafack, B. Ducharne and al, IEEE Trans. Mag., vol. 55, no. 7, 2019. [2] B. Ducharne, B. Gupta and al, IEEE Trans. on Mag., vol. 54, no. 11, 6202606, Nov. 2018. [3] A. Pulnikov, V. Permiakov and al, J. Magn. Magn. Mater., vol. 47, no. 9, p. 254–255, 2003. [4] K. S. H. Nguedjang, D. Y. A. Tene and al, J. Magn. Magn. Mater., pp. 1-10, 505, 166767, March 2020. [5] T. Yamaguchi, K. Senda and al, J. Physique IV, vol. 8, p. 717–20, 1998. [6] K. Senda, M. Ishida and al, Electr. Eng. Japan, vol. 126, p. 942–9, 1999.

Electromagnetic Modelling of the Magnetic Needle Probe Method from Parallel Domain Structure by FD Approximation

A technique to measure the full magnetic torque vector (three orthogonal torque components) on micro- and nano-scale magnetic materials is introduced. Measurements of a single axis or component of torque are most common and are very useful for hysteresis measurements of thin film structures in particular, where high shape anisotropy yields a near-proportionality of in-plane magnetic moment and the magnetic torque along the perpendicular in-plane axis. More generally, any component of cross-product torque involves a linear combination of perpendicular moment and magnetic susceptibility, yielding the rotational magnetic anisotropy or stiffness of the spin texture in response to torque. The method is demonstrated using a modified, single-paddle silicon-on-insulator resonant torque sensor [1]. The torsion mechanical susceptibilities to x- and z-torques are maximized by clamping the sensor at a single point. Figure 1 shows a completed device supporting a permalloy / cobalt oxide bilayer disk, deposited on a silicon paddle which is supported by a single beam. Mechanically-resonant AC torques are driven by an RF field containing a frequency component for each fundamental torsional mode of the device, and the resulting displacements read out through optical position-sensitive detection. A typical hysteresis measurement obtained as an in-plane DC bias field is swept is shown in Figure 2. The measurements are compared with micromagnetic simulations of the mechanical torque to verify the interpretation of the signals. As an application example, simultaneous observations of hysteresis in the net magnetization along with the field-dependent in-plane anisotropy is highly beneficial for studies of exchange bias.References: [1] Z. Diao et al., J. Vac. Sci. Technol. B., Vol. 31, p.051805 (2013)

Mechanical Torque Vector Measurements for Micromagnets

In the previous two decades, important technological advancements have expanded the range of temporal resolution in transmission electron microscopes (TEM). Commercial direct-counting and single-electron detectors have revealed dynamics in the ms-timescale. Laser-actuated photoemission microscopes [1, 2] combined with beam scanning, spatially-parsed large area detectors [3], and sparse-sensing algorithms [4], can now unlock phenomena at the ms to sub-ps timescales. Further optimization of the photoemission stage [5] and beam bunching technologies could potentially extend the temporal resolution into the deep fs-regime. Following our earlier concept paper [6], we now present the modifications to a pair of commercial instruments – one Schottky (200 keV) [7] and one thermionic (300 keV) [8] that can confer temporal information spanning the ns and ps range with MHz to GHz repetition rates, in the stroboscopic mode without an excitation laser. The key enabling technology is a pair of broadband phase-matched modulating and demodulating RF pulsers. We have demonstrated 11 ps and 30 ps on the 200 keV and 300 keV microscopes respectively. The placement of the pulsers, mounted immediately below the gun, allows for the preservation of all optical configurations otherwise available to the unmodified instrument, and therefore makes these instruments dual-mode, both stroboscopic time-resolved (strobe) mode and conventional continuous waveform (CW) mode. To show that the modifications preserved imaging and diffraction functionalities of the instrument, we obtained Au images and diffraction patterns using both a continuous and a strobed beam. We will also show the first proof-of-principle demonstration of these new instruments through images of RF waves moving though an interdigitated MEMS device.References: [1] VA Lobastov, R Srinivasan, AH. Zewail, Proc. Natl. Acad. Sci. 102 (2005) 7069−7073. [3] T LaGrange, et. al., Appl. Phys. Lett. 89 (2006) 044105 [3] T LaGrange, BW Reed, DJ. Masiel, MRS Bulletin 40 (2015) 22-28 [4] A Stevens, et al., Advanced Structural and Chemical Imaging 1 (2015). [5] DA Plemmons and DJ Flannigan, Chemical Physics Letters 683 (2017) 186–192 [6] J Qiu, et. al., Ultramicroscopy 161 (2016) 130. [7] C Jing, et al., Ultramicroscopy, 207 (2019) 112829. [8] JW Lau, et. al., Review of Scientific Instruments, 91 (2020) 021301. https://doi.org/10.1063/1.5131758 [*] We are grateful for the invaluable assistance from JEOL USA. This work was supported by DOE BES SBIR program Grant no. DE-SC0013121 and NIST award SB1341-16-CN-0035. During this work, K. Schliep was supported by the Research Associateship Program of the National Research Council and M. Katz was partially supported by the Professional Research Experience Program at the University of Maryland. Work at BNL was supported by the US DOE-BES, MSED, under Contract No. DESC0012704.

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Effect of Field Orientation and Infill Percentage on the VSM calibration factor of FFM 3D printed samples

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Observation of magnon-polarons in a uniaxial antiferromagnetic insulator Cr2O3

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