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Topological spin textures, such as skyrmions, have attracted intense interest in recent years. Magnetic skyrmions have been studied almost exclusively in bulk ferromagnets (FM) or FM multilayers. Antiferromagnets (AF) have also been predicted to harbor topological spin textures such as AF skyrmions. Topological Hall effect has been a primary indicator of spin textures in magnetic materials. We observe unambiguous evidence of topological Hall effect in Pt/Cr2O3 bilayers grown on Al2O3(0001) and Al2O3(11-20), where Cr2O3 epitaxial film is an antiferromagnetic insulator[1]. Although Cr2O3 is insulating, the topological magnetic textures can be detected through a novel phenomenon: “spin-Hall topological Hall effect” (SH-THE), similar to what recently observed topological Hall effect in Pt/Tm3Fe5O12 bilayers[2]. The Pt/Cr2O3 bilayers exhibit clear topological Hall resistivity for Cr2O3 thicknesses below 6 nm near and above room temperature, which is above the Néel temperature of Cr2O3, revealing the key role of thermal fluctuations in the formation of spin textures[3]. The similarity of topological Hall signals in (0001) and (11-20)-oriented Cr2O3 films indicates that the emergence of spin textures is insensitive to crystalline orientation. This first observational evidence of topological Hall effect in HM/AFI bilayers significantly expands our materials base to include the large family of AF insulators for the exploration of AF-based skyrmion technology.References: [1]. Yang Cheng, Sisheng Yu, Menglin Zhu, Jinwoo Hwang and Fengyuan Yang, “Evidence of Topological Hall Effect in Pt/Antiferromagnetic-Insulator Bilayers,” Phys. Rev. Lett. 123, 237206. [2]. A. S. Ahmed, A. J. Lee, N. Bagués, B. A. McCullian, A. M. A. Thabt, A. Perrine, P.-K. Wu, J. R. Rowland, M. Randeria, P. C. Hammel, D. W. McComb, and F.. Y. Yang, “Spin-Hall topological Hall effect in highly tunable Pt/ferrimagnetic-insulator bilayers,” Nano Lett., 19, 5683 (2019). [3]. Wenbo Wang, Matthew W Daniels, Zhaoliang Liao, Yifan Zhao, Jun Wang, Gertjan Koster, Guus Rijnders, Cui-Zu Chang, Di Xiao and Weida Wu, &quot;Spin chirality fluctuation in two-dimensional ferromagnets with perpendicular magnetic anisotropy&quot; Nat. Mater. 2019, 18, 1054.

MMM 2020

Evidence of Topological Hall Effect in Pt/Antiferromagnetic-Insulator Bilayers

The 65th Annual Conference on Magnetism and Magnetic Materials (MMM 2020) was held in a virtual form. The COVID-19 pandemic, with its associated uncertainty about international travel and the ability to gather in large groups, meant that the Steering Committee decided to cancel the face-to-face meeting that had been planned in Palm Beach, Florida November 2-6, 2020.

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Topological spin textures, such as skyrmions, have attracted intense interest in recent years. Magnetic skyrmions have been studied almost exclusively in bulk ferromagnets (FM) or FM multilayers. Antiferromagnets (AF) have also been predicted to harbor topological spin textures such as AF skyrmions. Topological Hall effect has been a primary indicator of spin textures in magnetic materials. We observe unambiguous evidence of topological Hall effect in Pt/Cr2O3 bilayers grown on Al2O3(0001) and Al2O3(11-20), where Cr2O3 epitaxial film is an antiferromagnetic insulator[1]. Although Cr2O3 is insulating, the topological magnetic textures can be detected through a novel phenomenon: “spin-Hall topological Hall effect” (SH-THE), similar to what recently observed topological Hall effect in Pt/Tm3Fe5O12 bilayers[2]. The Pt/Cr2O3 bilayers exhibit clear topological Hall resistivity for Cr2O3 thicknesses below 6 nm near and above room temperature, which is above the Néel temperature of Cr2O3, revealing the key role of thermal fluctuations in the formation of spin textures[3]. The similarity of topological Hall signals in (0001) and (11-20)-oriented Cr2O3 films indicates that the emergence of spin textures is insensitive to crystalline orientation. This first observational evidence of topological Hall effect in HM/AFI bilayers significantly expands our materials base to include the large family of AF insulators for the exploration of AF-based skyrmion technology.References: [1]. Yang Cheng, Sisheng Yu, Menglin Zhu, Jinwoo Hwang and Fengyuan Yang, “Evidence of Topological Hall Effect in Pt/Antiferromagnetic-Insulator Bilayers,” Phys. Rev. Lett. 123, 237206. [2]. A. S. Ahmed, A. J. Lee, N. Bagués, B. A. McCullian, A. M. A. Thabt, A. Perrine, P.-K. Wu, J. R. Rowland, M. Randeria, P. C. Hammel, D. W. McComb, and F.. Y. Yang, “Spin-Hall topological Hall effect in highly tunable Pt/ferrimagnetic-insulator bilayers,” Nano Lett., 19, 5683 (2019). [3]. Wenbo Wang, Matthew W Daniels, Zhaoliang Liao, Yifan Zhao, Jun Wang, Gertjan Koster, Guus Rijnders, Cui-Zu Chang, Di Xiao and Weida Wu, "Spin chirality fluctuation in two-dimensional ferromagnets with perpendicular magnetic anisotropy" Nat. Mater. 2019, 18, 1054.

poster

We have investigated various electronic transport properties such as the anisotropic magnetoresistance, planar Hall effect, and anomalous Hall effect in kagome Fe3Sn2, which has been predicted to be a type II Weyl metal. Based on magnetortransport, we determine the spin reorientation transition to peak at 120 K and coexistence of both out of plane and in plane phases at temperatures around the spin reorientation, indicative of a first order phase transition. In planar Hall effect, we discover a field antisymmetric contribution in addition to the standard field symmetric contribution. This field antisymmetric planar Hall effect has an in-plane 3-fold rotational symmetry, which is distinctively different from the symmetric counterpart. Furthermore, the temperature and field dependence of the field antisymmetric contribution is different from both the symmetric planar Hall effect and anomalous Hall effect, pointing to a different origin. A linear and antisymmetric planar Hall effect is predicted to be present in the case of non-magnetic Weyl semimetals. The experimental signatures in our case fit well with the prediction in addition to reflecting contributions from its ferromagnetism. As the magnetization of Fe3Sn2 has a 3-fold rotational degeneracy, the associated band structure and Weyl nodes determined by the magnetization direction owing to the spin-orbit coupling will have accordingly a 3-fold rotational degeneracy giving rise to the 3-fold antisymmetric PHE. We thus propose that the antisymmetric PHE that we discovered is the realization of an antisymmetric and linear planar Hall effect due to the presence of Weyl nodes near the Fermi level in a time reversal symmetry broken system. Our finding offers a promising route for macroscopically probing Weyl systems.References: [1] Neeraj Kumar, Y. Soh, Yihao Wang, et al., Anomalous planar Hall effect in a kagome ferromagnet, arXiv:2005.14237 (2020). [2] Nandy, S., G. Sharma, A. Taraphder, et al., Chiral Anomaly as the Origin of the Planar Hall Effect in Weyl Semimetals. Phys Rev Lett, 119(17): p. 176804 (2017). [3] M. Yao, H. Lee, N. Xu, et al., Switchable Weyl nodes in topological Kagome ferromagnet Fe3Sn2, arXiv:1810.01514 (2018).

Anomalous planar Hall effect in predicted type II Weyl Fe3Sn2

YbPtBi is a half Heusler alloy with claimed properties of topological Weyl nodes and chiral anomaly; antiferromagnetism from the RKKY coupling of localized Yb f-electrons at low temperatures; and heavy fermion behaviour as those localized f-electrons interact with the conduction bands [1,2]. So far only bulk crystals have been grown of YbPtBi with no published work on thin films. By using c-plane sapphire the half Heusler alloy has an epitaxially relationship of YbPtBi(111)||Al2O3(0001) and YbPtBi(110)||Al2O3(1100). With thin films we could have to option of induced strain, device fabrication and many other thin films manipulation techniques. In this work, we present a study of epitaxially grown YbPtBi thin films that grew as triangular islands with matched faceted edge orientations. The structure is confirmed to be epitaxial from x-ray diffraction and cross-sectional transmission electron microscopy. We also measure the electrical transport properties and find a non-metallic ρ(T) similar to other semimetals RePtBi (Re=Gd, Ce, Sm) half Heusler Alloy, although different from bulk YbPtBi. We measured a negative longitudinal magnetoresistance and the temperature dependence of an apparent chiral anomaly (Fig: a,b). Both of which are indicators of a possible Weyl semimetal state. We also obversed a large hysteretic MR at very low temperatures, 250 mK, not previously seen in YbPtBi.References: [1] C. Y. Guo, F. Wu, Z. Z. Wu, M. Smidman, C. Cao, A. Bostwick, C. Jozwiak, E. Rotenberg,Y. Liu, F. Steglich, and H. Q. Yuan, Nature Communications. 9, 4622 (2018) [2] B. G. Ueland, A. Kreyssig, E. D. Mun, J. W. Lynn, L. W. Harriger, D. K. Pratt, K. Prokeš, Z. Hüsges, R. Toft-Petersen, S. Sauerbrei, S. M. Saunders, Y. Furukawa, S. L. Bud’ko, R. J.McQueeney, P. C. Canfield, and A. I. Goldman, Phys. Rev. B. 99, 184431 (2019)

Epitaxial Growth Of The Weyl Semimetal YbPtBi (111) On C-plane Sapphire By Co-Sputtering

The magnetic properties of van der Waals magnetic topological insulators MnBi2Te4 and MnBi4Te7 are investigated by magneto-transport measurements. We evidence that the relative strength of the inter-layer exchange coupling J to the uniaxial anisotropy K controls a transition from an A-type antiferromagnetic order to a ferromagnetic-like metamagnetic state. A bi-layer Stoner-Wohlfarth model allows us to describe this evolution, as well as the typical angular dependence of specific signatures, such as the spin-flop transition of the uniaxial antiferromagnet and the switching field of the metamagnet. In micron-size magnets, the single-domain switching-field astroid are however partly truncated by the nucleation of domain walls along the easy-axis direction.References: A. Tan, V. Labracherie, N. Kunchur, A. U. B. Wolter, J. Cornejo, J. Dufouleur, B. Büchner, A. Isaeva and R. Giraud Metamagnetism of Weakly Coupled Antiferromagnetic Topological Insulators. Phys. Rev. Lett. 124, 197201. (2020)

Meta-Magnetism of Weakly-Coupled Antiferromagnetic Topological Insulators

The rare earth nitride series of intrinsic ferromagnetic semiconductors offers a rich selection of spin-orbit systems in which to study electrical transport and magnetic phenomenon, the various Hall effects being one of the many meeting places of these[1,2]. The central member of the series GdN (8S7/2) has a strong spin only magnetisation and relatively simple band structure, dominated by the Gd 5d conduction band and N 2p valence band. Electron doping is routinely achieved via the inclusion of nitrogen vacancies. Here we report on 'anomalous' Hall effect data in heavily doped GdN, which show an apparent change of sign of the dominant charge carrier as the sample is cooled through the ferromagnetic transition, while the anomalous Hall effect retains the negative sign of electron doped GdN. We will discuss these in the context of the calculated band structures of stoichiometric and heavily doped GdN.References: [1] W. F. Holmes-Hewett, R. G. Buckley, B. J. Ruck, F. Natali and H. J. Trodahl, 4f conduction in the magnetic semiconductor NdN, Phys. Rev. B. 100, 195119 (2019) [2] W. F. Holmes-Hewett, F. H. Ullstad, B. J. Ruck, F. Natali and H. J. Trodahl, Anomalous Hall effect in SmN: Influence of orbital magnetism and 4f band conduction, Phys. Rev. B. 98, 235201 (2018)

Anomalous Hall effects in rare earth nitrides

Spin polarization in nonmagnetic materials originates from the break of inversion crystalline symmetry that could occur globally or locally. Centrosymmetric (CS) nonmagnetic materials with hidden spin polarization induced by non-CS site symmetries and spin-orbit coupling are promising candidates for spintronic applications, in light of the zero net spin polarization and modulatable spin effects hidden in the local structures. There is, however, an open issue regarding the possible spin splitting induced by broken inversion symmetry at the sample surface. Therefore, it is critical to perform combined experimental and theoretical studies on centrosymmetric TMDC materials such as 2H-MoTe2 to explore the mechanism of the hidden spin polarization. 2H-MoTe2 crystallizes in a trigonal prismatic arrangement with an in-plane lattice constant of 3.517 Å and an out-of-plane lattice constant of 13.962 Å. The unit cell of it is centrosymmetry, but the monolayer has non-centrosymmetric structure. With the virtue of low detection depth of spin-ARPES (<6 Å with He-I), a large spin splitting of 236 meV and opposite spin polarizations up to 80% along out-of-plane direction (z axis) in K and K′ valleys were observed, consist with the density functional theory (DFT) calculations. We further found from the DFT calculations that a medium dipole field mimicked the surface symmetry breaking in ARPES measurements induces negligible variation of spin polarization, confirming that the measured spin effects originate from the intrinsic hidden spin polarization in 2H-MoTe2. The large spin splitting and net spin polarization found in spin-ARPES experiments also suggest that the hidden spin effects in inversion symmetric layered compounds can be used to generate large spin splitting on the surfaces in the absence of strong dipole field. Our combinatorial experimental and theoretical studies clarify the existence of hidden spin polarization in the centrosymmetric materials and opens the way of designing novel functional materials with coexisting hidden spin polarization and other hidden effects, such as hidden orbital polarization and hidden Berry curvature, for the energy efficient spintronics applications.

Direct observation of hidden spin polarization in 2H-MoTe2

Magnetic impurities in metals spin polarize their surroundings. This Ruderman-Kittel-Kasuya-Yosida (RKKY) polarization has been fundamental in the understanding of interactions in magnetic atoms and layers. When the impurity is heavy and magnetic, its large atomic spin-orbit coupling unquenches the orbital momentum. This is the case of lanthanide atoms, which have a significant orbital momentum responsible for their strong magnetocrystalline anisotropy. Recent utilization of this atomic spin-orbit coupling in spintronics include the perpendicular magnetic anisotropy of thulium iron garnet (TIG) films [1-4], the voltage-controlled magnetic anisotropy of interfacial rare-earth ions [5-6], and double compensation points of ferrimagnets [7]. In this presentation, we study lanthanide impurities in simple metals. The lanthanide orbital momentum couples to conduction electrons via the so-called skew scattering and induces a rotational current [8]. The predicted current has an orbital momentum density very similar to the RKKY one, with an algebraic decay and oscillations at twice the Fermi wavenumber. In addition to the charge density profile, we compute the observable effects, namely the Oersted magnetic field and Knight shift.References: [1] M. Kubota, A. Tsukazaki, F. Kagawa, K. Shibuya, Y. Tokunaga, M. Kawasaki, and Y. Tokura, APEX 5, 103002 (2012). [2] C. Tang, P. Sellappan, Y. Liu, Y. Xu, J. E. Garay, and J. Shi, Phys. Rev. B 94, 140403(R) (2016). [3] C. N. Wu, C. C. Tseng, Y. T. Fanchiang, C. K. Cheng, K. Y. Lin, S. L. Yeh, S. R. Yang, C. T. Wu, T. Liu, M. Wu, M. Hong, and J. Kwo, Sci. Rep. 8, 11087 (2018). [4] C. O. Avci, A. Quindeau, C.-F. Pai, M. Mann, L. Caretta, A. S. Tang, M. C. Onbasli, C. A. Ross, and G. S. D. Beach, , Nat. Mat. 16, 309 (2017). [5] A. O. Leon, A. B. Cahaya, and G. E. W. Bauer, Phys. Rev. Lett. 120, 027201 (2018). [6] AO Leon, GEW Bauer, accepted by Journal of Physics: Condensed Matter. [7] M. Imai, H. Chudo, M. Ono, K. Harii, M. Matsuo, Y. Ohnuma, S. Maekawa, and E. Saitoh, Appl. Phys. Lett. 114, 162402 (2019). [8] A. B. Cahaya, A. O. Leon, M. Rahimi Aliabad, G. E. W. Bauer, arXiv:2006.13024

Rotational currents around lanthanide dopants in simple metals

The signature of magnetism without having a ferromagnet in the sample stack is both novel and fascinating from fundamental research point of view. It is possible to alter the electronic states of non-ferromagnetic materials (Cu, Mn, Sc, Pt) to overcome the Stoner criterion and make them ferromagnetic at room temperature1,2. In this context it is desired to quantify the magnetic moment at the interface of such non-FM/OSC. We have studied the Cu/C60 heterostructure and quantified the magnetic moment induced in Cu using X-ray magnetic circular dichroism (XMCD) sum rules. The multilayer of Cu/C60 were prepared on Si (100) substrate without breaking the vacuum using DC magnetron sputtering and thermal evaporation for Cu and C60, respectively. SQUID magnetometry on sample S1:(Si(100)/Ta(5nm)/C60(8nm)/Cu(1.8nm)/C60(4nm)/Ta(2nm)) and S2:(Si(100)/Ta(5nm)/C60(16nm)/[Cu(1.8nm)/C60(8nm)]x2/Ta(2nm)) exhibit a clear ferromagnetic hysteresis even in the absence of any ferromagnetic element in the sample stack. The induced magnetic moment in the samples is corroborated to the charge transfer and the molecular coupling between the metal (Cu) and carbon. The origin of the charge state of C60 to a reconstructed interface is due to (4 4) 7-atom vacancy holes in the surface3. The possible reason of this induced magnetic moment is hybridization between dcu and pC60 orbitals1. In order to evaluate the spinterfacial magnetic moment, XMCD has been performed on the samples. Figure1 shows the XAS and XMCD spectra of the samples. The XAS spectra do not exactly match with Cu. The reason behind such misalignment is the hybridization between Cu and C60. Due to the charge transfer at the reconstructed Cu/C60 interface the density of state of Cu has been modified and exhibits ~ 0.01 μB /atom magnetic moment4. Our understanding of the interface between the NM/OSC heterostructures may bring the new insights to the field of organic spintronics.References: 1. F. Al Ma'Mari et.al., Nature 524, 69 (2015). 2. F. Al Ma’Mari et al., PNAS, 1620216114 (2017). 3. W.W.Pai et.al., PRL 104, 036103 (2010). 4. P. Sharangi et al., (unpublished)

Quantifying induced moment in non-magnetic Cu – C60 interfaces via x-ray magnetic circular dichroism

Mn-Ga alloys show promise for spintronic applications based on their tunable saturation magnetization (Ms) and goldilocks region perpendicular magnetic anisotropy (Ku).1 Thin films with perpendicular magnetic anisotropy have potential as low-dimensional highly reliable spintronic devises.2-5 The task remains to optimize magnetic properties for applications as a function of composition and dimensionality. In this study we attempt to understand the impact of composition on magnetic properties of Mn-Ga systems in the D022 structure. Density Functional Theory (DFT) calculations are used to study the role of vacancies on Ms and Ku of Mn-Ga family of alloys. While the DFT calculations capture the general trends seen in experiments, they are unable to quantitatively predict Ms and Ku with sufficient accuracy. This is attributed to the inherent complexities in the thin film growth of Mn-Ga systems, where the variations in Ms and Ku show a strong dependence on the growth variables. Machine Learning (ML) is implemented as a low-cost alternative to DFT, where we train and validate data-driven models based on Ms and Ku data compiled from surveying experimental literature. The ML models enable rapid predictions of Ms and Ku for previously unexplored compositions. New compositions are identified with implications in emerging spintronics applications.References: 1) H. Kurt, K. Rode, M. Venkatesan, P. Stamenov, PHYSICAL REVIEW B 83, 020405(R) (2011) 2) S. Iwasaki and K. Ouchi, IEEE Trans. Magn. 14, 849 (1978) 3) P. F. Carcia, J. Appl. Phys. 63, 5066 (1988) 4) T. Seki, T. Shima, K. Takanashi, Y. Takanashi, E. 82, 2461 (2003) 5) S. N. Piramanayagam, J. Appl. Phys. 102, 011301 (2007).

Density Functional Theory and Machine Learning Guided Study of Mn-Ga Alloys with Targeted Magnetic Properties

How strong correlations drive quantum states of matter with nontrivial topology is an outstanding issue in contemporary condensed matter physics. This talk will provide an overview and discuss the latest development on Weyl-Kondo semimetal, which has been concurrently advanced by theoretical [1,2] and experimental [3,4,5] studies. The theoretical work addressed a nonsymmorphic Anderson lattice model that breaks the inversion symmetry while preserving the time-reversal symmetry, whereas the experimental effort focused on the non-magnetic non-centrosymmetric and non-symmorphic heavy fermion semimetal Ce3Bi4Pd3. The salient signatures of the Weyl-Kondo semimetal include a correlation enhanced specific heat C=ΓT3 [3], and a giant zero-magnetic-field Hall response and even-in-field Hall effects [4]. The latest high magnetic field experiments observed a two-stage topological phase transition, from Weyl-Kondo semimetal to Kondo insulator to heavy-fermion metal [5]. To bridge the latest experiments and our theoretical work, we investigated the aforementioned Anderson lattice model in the presence of a Zeeman coupling. Tuning both the Zeeman coupling and the inversion-symmetry-breaking potential controls the position and number of Weyl nodes in the Brillouin zone, and several topologically distinct phases emerge in this model.References: [1] H.-H. Lai, S. E. Grefe, S. Paschen, and Q. Si, Proc. Natl. Acad. Sci. U.S.A. 115, 93 (2018). [2] S. E. Grefe, H.-H. Lai, S. Paschen, and Q. Si, Phys. Rev. B, 101, 075138 (2020). [3] S. Dzsaber, L. Prochaska, A. Sidorenko, G. Eguchi, R. Svagera, M. Waas, A. Prokofiev, Q. Si, and S. Paschen, Phys. Rev. Lett. 118, 246601 (2017). [4] S. Dzsaber, X. Yan, G. Eguchi, A. Prokofiev, T. Shiroka, P. Blaha, O. Rubel, S. E. Grefe, H.-H. Lai, Q. Si, and S. Paschen., arXiv preprint arXiv:1811.02819, (2018). [5] S. Dzsaber, D. A. Zocco, A. McCollam, F. Weickert, R. McDonald, M. Taupin, X. Yan, A. Prokofiev, L. M. K. Tang, B. Vlaar, et al., arXiv preprint arXiv:1906.01182 (2019).

Weyl-Kondo Semimetals: Correlated Topology and Control of Nodes INVITED

Magnon spin Nernst effect (SNE) has recently been proposed as a bulk effect in antiferromagnetic insulators without considering diffusions and boundaries1,2. However, real experiments3 deal with situations far from the ideal bulk picture in that: 1) the system is finite and shares imperfect boundaries with the detecting leads; 2) both the electrons in the leads and the magnons are diffusive; 3) the thermal power rather than the temperature gradient is calibrated. To properly accommodate these complexities, we formulate a diffusive theory of the SNE of antiferromagnetic magnons under a realistic device geometry. By solving the coupled spin diffusion equations of magnons and electrons with a finite spin transmission across the boundaries, we find that the detectable signal can be much larger than that predicted by the bulk picture. The diffusive effects also lead to a different phase diagram of the SNE compared to the bulk theory without diffusion. Counterintuitively, we also find that the diffusive magnon SNE exhibits an even symmetry with respect to a perpendicular magnetic field.References: 1. R. Cheng, S. Okamoto and D. Xiao, Phys. Rev. Lett., Vol. 117, 217202 (2016) 2. V. A. Zyuzin and A. A. Kovalev, Phys. Rev. Lett., Vol. 117, 217203 (2016) 3. Y. Shiomi, R. Takashima and E. Saitoh, Phys. Rev. B, Vol. 96, 134425 (2017)

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Evidence of Topological Hall Effect in Pt/Antiferromagnetic-Insulator Bilayers

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