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Unidirectional spin Hall magnetoresistance (USMR) is a magnetoresistance effect with potential applications to read two-terminal spin-orbit-torque (SOT) devices directly. In this work, we observed a large USMR value (up to 0.710-11 per A/cm2, 50% larger than reported values from heavy metals) in sputtered amorphous PtSn4/CoFeB bilayers. Ta/CoFeB bilayers with interfacial MgO insertion layers are deposited as control samples. The control experiments show that increasing the interfacial resistance can increase the USMR value, which is the case in PtSn4/CoFeB bilayers. The observation of a large USMR value in an amorphous spin-orbit-torque material has provided an alternative pathway for USMR application in two-terminal SOT devices.&lt;br&gt;

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MMM 2022

Observation of unidirectional spin Hall magnetoresistance in amorphous PtSn4/CoFeB bilayers

Unidirectional spin Hall magnetoresistance (USMR) is a magnetoresistance effect with potential applications to read two-terminal spin-orbit-torque (SOT) devices directly. In this work, we observed a large USMR value (up to 0.710-11 per A/cm2, 50% larger than reported values from heavy metals) in sputtered amorphous PtSn4/CoFeB bilayers. Ta/CoFeB bilayers with interfacial MgO insertion layers are deposited as control samples. The control experiments show that increasing the interfacial resistance can increase the USMR value, which is the case in PtSn4/CoFeB bilayers. The observation of a large USMR value in an amorphous spin-orbit-torque material has provided an alternative pathway for USMR application in two-terminal SOT devices. 

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poster

#### Welcome to the 67th Annual Conference on Magnetism and Magnetic Materials, MMM 2022!

The Conference was held from October 31 to November 4 and offers both in-person and on-demand content.

MMM 2022 is sponsored jointly by AIP Publishing and the IEEE Magnetics Society. Members of the international scientific and engineering communities interested in recent developments in fundamental and applied magnetism are invited to attend and contribute to the technical sessions. The technical program will include invited and contributed papers in oral and poster sessions, invited symposia, a tutorial, and several special sessions. This Conference provides an outstanding opportunity for worldwide participants to meet their colleagues and collaborators and discuss developments in all areas of magnetism research.

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L10-ordered MnAl, a perpendicularly magnetized film material, has attracted much attention due to its high magnetic anisotropy, low saturation magnetization, and low magnetic damping for spin-transfer-torque magnetic random access memory (STT-MRAM) applications. However, in magnetic tunnel junctions (MTJs) with a single MnAl ferromagnetic layer, the TMR ratio has not been confirmed. This is due to the large lattice mismatch between MgO tunneling barrier and MnAl layer, which prevents the coherent tunneling of Δ1 electrons (1). In this work, we utilized Co-doped MnAl and MgAl2O4 tunneling barrier to reduce lattice mismatch and inserted a very thin Fe layer into (MnCo)Al/MgO interface to improve TMR effect.
The structure of the MTJs prepared in this study is shown in Fig.1. The MTJ films were prepared using the ultrahigh vacuum magnetron sputtering method. (MnCo)Al layers with low roughness and high (001) orientation by adding 2% Co. The composition of MgAl2O4 was measured using X-ray photoelectron spectroscopy (XPS). Compositional analysis showed that the composition of MgAl2O4 was Mg : Al : O =9.2 : 18.9 : 41.5 (atom%). MTJ devices were microfabricated and characterized their TMR properties by DC 4-probe method.
We succeeded in observing a TMR ratio of 8% at 300K without an insertion layer by using (MnCo)Al electrode and MgAl2O4 tunneling barrier as shown in Fig. 2(a). In addition, TMR ratio was improved to 9.4% by insertion of ultra-thin Fe layer into the (MnCo)Al/MgO interface as shown in Fig. 2(b). This translates to 18.8% in terms of magnetization parallel state. Since the RA product was decreased from 1.2 MΩμm2 to 223 kΩμm2 by insertion of Fe, coherent tunneling process was thought to be promoted by the interfacial modification.
This work was supported by the Center for Advanced Spintronics Research and Development, the Center for Spintronics Cooperative Research and Education and Development, and the Center for Spintronics Cooperative Research and Education, Tohoku University. 

**References:** 
(1) H.Saruyama, M.Oogane, Y.Ando, 2013, Jpn. J. Appl. Phys., 52, 063003 

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Dependence of TMR and RA on Fe insertion layer thickness in MTJs using L10 (MnCo)Al electrode and MgAl2O4 insulating layer

Magnetoresistive sensors have been enthusiastically selected for applications requiring magnetic field detection with sensors combining small footprint (1), highly linear response curves with low coercivity and low field detectivities. From the viable alternatives (2), MgO-based magnetic tunnel junctions (TMR) offer very competitive performance values, as sensitivity as large as 300 %/mT are reported (3). The optimization of the sensor response includes using soft magnetic free layers, based on CoFeB and NiFe alloys (4).
Here we report the performance of TMR sensors including CoFeBTa and CoFeBSi soft magnetic films as free layers (FL). Magnetic tunnel junction stacks based on (Ta 5/Ru 10)x3/Ta 5/Ru 5/MnIr 8/CoFe 2.2/Ru 0.65/CoFeB 2/MgO/CoFeB/FL2/cap (nm) (fig. 1) were grown on 200 mm wafers using a combination of ion beam and magnetron sputtering deposition from the 14 targets available in the machine. The TMR stacks were magnetically characterized by vibrating sample magnetometry and CIPT, while microfabricated devices (rectangular shaped pillars of varying areas and aspect ratios) were evaluated for transfer curve sensitivity, linear range and noise.
The magneto-crystalline anisotropy, Hk, was assessed for CoFeBTa and CoFeBSi films, with values of 2.1 and 5.3 mT measured for 4 nm films integrated in the TMR stacks. Although these values are larger than for single NiFe FL (1.7 mT)(fig. 2), the global performance of the CoFeBTa/CoFeBSi-based sensors is improved, with magnetoresistance of 210 %, when comparing with 190 % (CoFeB) or 150 % (NiFe). Field sensitivities up to 80 %/mT are obtained, with similar hysteresis (Hc) as for CoFeB or NiFe stacks.
The low frequency noise (1/f dominated) characteristic was evaluated for the microfabricated devices. As an example, sensors with FL2 = CoFeBTa (10 TMR elements connected in series) provided Hooge factor αH = 2.4x10-10 μm2 and detectivity levels of D = 4.5 nT/√Hz at 10 Hz. These values are aligned with previously reported values with similar materials (4).
Acknowledgments: FCT grant UI/BD/151461/2021 

**References:** 
(1) M. Silva, D.C. Leitão, S. Cardoso and P. P. Freitas, IEEE Trans. Magn. 53, 7762720 (2017) 
(2) C. Zheng et al., IEEE Trans. Magn. 55-4, pp. 1-30 (2019) 
(3) TMR9001, MultiDimension Technology, Datasheet available online: http://www.dowaytech.com/en/1866.html (accessed on 24 June 2022) 
(4) M. Rasly et al., J. Phys. D: Appl. Phys. 54, 095002 (2021) 

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CoFeBX layers for MgO based magnetic tunnel junction sensors with improved noise and detectivity

Spintronics-based devices offer certain key advantages like ease of fabrication with Si-substrate, non-volatile memory, low operational voltage, and non-linear device characteristics. Hardware security is a research domain that heavily relies on CMOS-based ICs, and the defense and attack mechanism is developed accordingly.
In this work, we explore shape anisotropy-based PMA Double barrier MTJ based on Verilog-A behavioral model (1) to design a possible Logic locking (2) system for Hardware Security. Logic Locking is a widely used security mechanism to counter multiple threats (3). Due to larger free layer thickness, the s-PMA DMTJ has better thermal stability even in the sub-10nm dimension. The current work focuses on Logic locking applications using this device, analyze its behavior under process variation in certain key parameters using Monte-Carlo simulations, and finally performs Eye-diagram performance analyses to test the design for high-speed digital logic applications. The results indicate that the s-PMA DMTJ has good thermal stability, smaller size (10nm dimension), robustness to device imperfections, and ability to work in high-speed digital circuits compared to other emerging MTJ structures such as STT MTJ, SOT MTJ, VG-SOT MTJ, etc.
Fig. 1(a) represents the block diagram of the logic Locking block, and Fig. 1(b) represents the circuit for implementing the desired operation. We have performed electrical simulations in TSMC 40nm CMOS generic process design kit using the cadence specter simulator with W/L ratio = 3, the temperature at 300K. Fig. 2(a) and 2(c) represent some circuit performance comparisons like the Eye-diagram test for high-speed circuits, and Table 1 presents the simulation data for the same. Fig. 2(b) shows that VG-SOT MTJ (4) fails the eye-diagram test for similar applications for comparison with s-PMA DMTJ. 

**References:** 
(1) H. Wang et al., “Modeling and Evaluation of Sub-10-nm Shape Perpendicular Magnetic Anisotropy Magnetic Tunnel Junctions,” IEEE Transactions on Electron Devices, vol. 65, no. 12, pp. 5537-5544, Dec. 2018. 
(2) H. M. Kamali, K. Z. Azar, F. Farahmandi, and M. Tehranipoor, “Advances in Logic Locking: Past, Present, and Prospects,” Cryptology ePrint Archive, 2022. 
(3) S. Bhunia, and M. Tehranipoor, “Hardware security: a hands-on learning approach,” 1st Edition, 2018. 
(4) K. Zhang, D. Zhang, C. Wang, L. Zeng, Y. Wang and W. Zhao, “Compact Modeling and Analysis of Voltage-Gated Spin-Orbit Torque Magnetic Tunnel Junction,” IEEE Access, vol. 8, pp. 50792-50800, 2020. 
(5) K. Watanabe et al., “Shape anisotropy revisited in single-digit nanometer magnetic tunnel junctions,” Nature Communication, 2018. 

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Double Barrier s PMA MTJ

With the rapid growth of technologies such as the Internet of Things (IoT) and artificial intelligence (AI) in recent years, giant data transmission and processing capacities of computers have faced major hurdles (1, 2). At the moment, memory is the key bottleneck in computer processing big data processes. The CPU and the memory are distinct in the standard Von Neumann design, while frequent data exchange uses a lot of energy, resulting in the "Memory Wall" problem (3). On-chip cache, being the crucial constituent of CPU, accounts for a pivoltal portion of the system's overall power consumption. If the power wastage of the on-chip cache could be lowered, the ultimate performance of the CPU can be strengthened. The typical SRAM-based cache is vulnerable to high static leakage power consumption, and scaling up its capacity is challenging. Magnetic random access memory (MRAM) (4), as a new non-volatile storage technology, is expected to break the limitation at the cache level (5).
In the paper, MRAM cache is used to limit static leakage power consumption. A quad-core CPU MRAM hierarchical cache system is established in the designed MRAM cache, with the high-speed Spin-Orbit-Torque (SOT)-MRAM (6) functioning as the L1 cache and the high-density Spin-Transfer-Torque(STT)-MRAM (7) serving as the L2 shared cache. A non-inclusive allocation method is adopted for the data-exchange strategy, by which the number of the write operation in the L2 STT-MRAM cache is reduced, and the energy consumption of the system is further reduced. The designed system is simulated and verified based on gem5 (8) software framework. The simulation results show that strategy of the hybrid MRAM memory is a promising candidate for high-speed and low-power on-chip cache. 

**References:** 
(1) Y. Li, Z. Wang, R. Midya et al., Journal of Physics D: Applied Physics., vol. 51, p.503002(2018) 
(2) J.-M. Hung, X. Li, J. Wu et al., IEEE Transactions on Electron Devices., vol. 67, p.1444-1453(2020) 
(3) X. Huang, C. Liu, Y.-G. Jiang et al., Chinese Physics B., vol. 29, p.078504(2020) 
(4) M. Durlam, P. J. Naji, A. Omair et al., IEEE Journal of Solid-State Circuits., vol. 38, p.769-773(2003) 
(5) F. Oboril, R. Bishnoi, M. Ebrahimi et al., IEEE Transactions on Computer-Aided Design of Integrated Circuits and Systems., vol. 34, p.367-380(2015) 
(6) K. Jabeur, L. D. Buda-Prejbeanu, G. Prenat et al., International Journal of Electronics Science and Engineering., vol. 7, p.501–507(2013) 
(7) D. Apalkov, A. Khvalkovskiy, S. Watts et al., ACM Journal on Emerging Technologies in Computing Systems., vol. 9, p.13:1–13:35, (2013) 
(8) N. Binkert, B. Beckmann, G. Black et al., ACM SIGARCH computer architecture news., vol. 39, p.1-7(2011) 

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Hierarchical Cache Configuration Based on Hybrid SOT and STT

Spin-transfer-torque magnetic random-access memory (STT-MRAM) is one of the promising emerging memory technologies as it offers high speed and non-volatility required for embedded applications such as SOCs, IOTs, and Microprocessors (1).However, due to the magnetic nature of the STT-MRAM, the free layer of the memory cell is sensitive to the external magnetic field and the thermal fluctuation (2). For the practical application scenarios of STT-MRAM, the memory may be exposed to high external magnetic field for short time. In this way, high immunity is required for the STT-MRAM memory to avoid any possible data errors caused by the external magnetic field.
In the paper, the memory model at array level is established to study the immunity property of STT-MRAM. By investigation on the magnetic field distribution of the memory array under different external magnetic field, the three operation modes, including standby, active read and active write modes, are simulated and analyzed. Based on the simulation results, the immunity property and the reliability of the memory array is discussed and optimized.
The paper is organized as follows. Firstly, the STT-MRAM array model is established in the HFSS. The magnetic field distribution in the memory array is simulated. The influences of the key geometrical parameters on the magnetic distribution, including the thicknesses of the epoxy and the electrode layer, are investigated. Secondly, to improve the immunity property of the memory, the approach of adding high permeability magnetic shield material is proposed in the paper. Thirdly, the influence of the magnetic immunity on the data reliability of the memory is investigated. The reliability is basically all about data retention and it is determined by effective Eb (3). And the bit error rates (BERs) of the MTJs under the states of standby, active read and active write, are also analyzed in the paper.
Fig.1 The established array model of the STT-MRAM for the immunity investigation. (a) The magnetic field distribution of STT-MRAM array. (b) The magnetic distribution in single STT-MRAM cell. 

**References:** 
(1) B. Bhushan, L. T. Guan, D. Shum et al., 2018 IEEE International Memory Workshop (IMW), p. 1-4, (2018). 
(2) S. Srivastava, K. Sivabalan, J. H. Kwon, et al. Applied Physics Letters, 114(17):172405. (2019). 
(3) T. Y. Lee, K. Yamane, L. Y. Hau, et al. 2020 IEEE International Reliability Physics Symposium (IRPS). p. 1-4 (2020). 

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High reliability of STT MRAM with enhanced magnetic immunity

Spin transfer torque magnetoresistive RAM (STT-MRAM) is one of the promising emerging memory technologies, with the merits of CMOS-compatibility, fast read speed, high density and non-volatile, etc. (1). However, the write speed is one of the major challenges for STT-MRAM, especially in high speed applications. For a reliable writing operation, high writing current and enough duration time are required, which could decrease the life-time of the tunnel layer in the MTJ device and cause extensive power consumption. So, the writing strategy of the STT-MRAM is one of the key issues in the memory design. Several writing strategies are proposed to improve the writing reliability, lower the power consumption, as well as increase the life-time of the device.
In the paper, the pipeline structure combined with the parallel shift register circuit is proposed to achieve the high write efficiency for the STT-MRAM. Figure 1 shows the block diagram of the proposed multi-bit parallel pipeline-circuit. In the designed circuit, the introduction of bit-parallel processing is essential to achieve high throughput operation (2).The parallel shift register circuit is added in the STT-MRAM to allow serial data to be transferred to the sensing circuit in parallel. Moreover, the pipeline structure is also utilized in the peripheral circuit. Several latches operating in response to a clock signal to process the data by dividing the write operation into a plurality of stages (3). Thus, the multi-bit parallel data can be carried out in pipelining manner, greatly increasing the average write speed and the throughput of STT-MRAM. The proposed write strategy of STT-MRAM achieves better write efficiency and high throughput, which has potential high speed application of STT-MRAM in the future.
Fig.1 The block diagram of the proposed multi-bit parallel pipeline-circuit design for STT-MRAM. 

**References:** 
(1) K. Huang, R. Zhao, N. Ning, et al., IEEE Trans. Circuits Syst., vol. 61, p. 2614-2623 (2014). 
(2) R. Kashima, I. Nagaoka, M. Tanaka, et al. IEEE Trans. Appl. Supercond., vol.99, p. 1-1 (2021). 
(3) Y. Ma, S. Miura, H. Honjo, et al., Jpn. J. Appl. Phys., vol. 59, p. SG (2020). 

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Novel multi bit parallel pipeline

Spintronic devices driven by spin-orbit torque (SOT) have a lot of potential for future neuromorphic computing hardware platforms. Nevertheless, problems such as multistate loss, weight time-dependent variability, and output discontinuity ensue when the device size is reduced to the nanoscale, which is contradictory to the needs of traditional high-precision neural networks. In this study, we propose a high-precision all-spin neural network based on magnetization switching of a simple nanoscale multi-functional SOT device. The all-spin neural network is implemented by the Binary Weight Network, in which binary synapse is encoded by the two states formed by the device's deterministic switching and the practical neuron is realized by its stochastic switching probability. Furthermore, we use a difference derivation training algorithm for the general-purpose network in a novel way to be more compatible with the discontinuous neuron output. Using this strategy, our network recognition accuracy can reach ~81.73% on the universal CIFAR-10 dataset, paving the way for the practical hardware implementation of nanoscale SOT devices in high-precision compact neuromorphic computing. 

**References:** 
J. Zhou, T. Zhao and J. Chen, Advanced Materials., Vol. 33, p.2103672 (2021) 
S. Zhang, J. Zhang and L.You, Science China Information Sciences., Vol. 65, p.1-9 (2022) 

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Binary weight network utilizing multi functional spin

We report the experimental demonstration of long-range orbital torques generated by Nb and Ru and detected by spin-torque ferromagnetic resonance (ST-FMR) measurements in Nb/Ni and Ru/Ni bilayers. We identify the orbital torques from the sign-reversal and a strong enhancement in the damping-like torque observed in Nb (Ru)/Ni bilayers as compared to Nb (Ru)/FeCoB bilayers as theoretically predicted1. The long-range nature of orbital transport in the ferromagnet was revealed by varying the thickness of Ni in Nb (Ru)/Ni bilayers which is markedly different compared to the regular spin absorption in the ferromagnet that takes place in the first few layers confirming the recent prediction2. Finally, we show that the external injection of orbital current in a heavy metal such as Pt can convert the orbital current into a spin-current leading to higher switching efficiency and the enhanced spin-current generation that could both be potentially attractive for the application3,4. 
**References** 1. Go, D. & Lee, H.-W. Orbital torque: Torque generation by orbital current injection. Phys. Rev. Res. 2, 013177 (2020).
2. Go, D. et al. Long-Range Orbital Magnetoelectric Torque in Ferromagnets. arXiv 2106.07928, 1–6 (2021).
3. Ding, S. et al. Harnessing Orbital-to-Spin Conversion of Interfacial Orbital Currents for Efficient Spin-Orbit Torques. Phys. Rev. Lett. 125, 177201 (2020).
4. Go, D., Jo, D., Lee, H.-W., Kläui, M. & Mokrousov, Y. Orbitronics: Orbital currents in solids. EPL (Europhysics Lett. 135, 37001 (2021).
5. 
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Detection of long range orbital torques

Within magnetic materials, anisotropic magnetoresistance (AMR) measures the dependence of the resistivity on the angle between the high magnetic susceptibility direction of the magnetic order and the current direction. When analyzed using spectral decomposition, the AMR of most magnetic materials is composed of even harmonics the most common of which are 2-fold (C2) and 4-fold (C4) arising from s-d scattering and crystal field effects respectively. The generation of odd harmonics in the spectral decomposition of the AMR are observed in magnetic films when the magnetic film is combined with another non-magnetic material to form a heterostructure. The observed unidirectional AMR is a result of the explicit breaking of the spatial inversion symmetry at the interface of the engineered heterostructure. Alternatively, the spatial inversion symmetry may be broken internally within the magnetic film under the application of a magnetic field leading to the observation of signatures of unidirectional AMR in the spectral decomposition without the presence of the non-magnetic material. In this work, we observe odd spectral harmonics (C1 and C3) associated with the presence of unidirectional AMR in 20 nm thin-films of antiferromagnetic FeRh measured at 20K, as seen in Fig. 1(A). In Fig. 1(B), the presence of the odd spectral harmonics is confirmed using a tight-binding representation of the tetragonal FeRh lattice in the antiferromagnetic phase where the transport quantities are calculated using the non-equilibrium Green’s function formalism. Furthermore, we attribute the presence of the C1 and C3 harmonics to the magnetic moment that the Rh atoms develop when immersed in an external in-plane magnetic field. We quantify the size of the inherent unidirectional AMR component as a function of the applied magnetic field and show that the internal unidirectional AMR component is non-negligible and omnipresent in AMR measurements even in the absence of non-magnetic layers. 
**References** J. Oh, L.Humbard, V. Humbert, AIP Advances 9, 045016 (2019)
T. Huong T. Nguyen, V.Nguyen, Communications Physics volume 4, Article number: 247 (2021)
 
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Intrinsic Unidirectional Anisotropic Magnetoresistance in Thin Film FeRh

Compensated ferrimagnets [1,2] with two inequivalent magnetic sublattices can exhibit finite spin polarization, anomalous Hall effect and tunneling magnetoresistance like a ferromagnet, even when the net magnetization exactly vanishes at the magnetic compensation point. This material class has attractive potential for high-density, ultrafast, and low-power spintronic applications. Cubic Mn2RuxGa (MRG) is a typical example of compensated ferrimagnet with high spin polarization and high tunability of compensation temperature by freely varying the Ru content x over a broad range (0.3 < x < 1.0) [3]. Here, we systematically studied MRG-based polycrystalline ingots prepared by arc melting, followed by annealing at 1073 K for seven days. We surprisingly found that, in equilibrium bulk form, the cubic structure is unstable when x < 0.75, which substantially reduces the tunability of MRG. We concluded that previously reported Ru-deficient MRG thin films are mostly metastable. At equilibrium, MRG can never compensate below ~350 K.
To overcome this limitation, we alloy MRG with a fourth element V, which helps to stabilize the cubic structure while providing less valence electron than Mn and Ru. We systematically investigate the Mn2Ru0.75VyGa quaternary system. Figure 1(a) shows the temperature dependence of magnetization M(T) measured with a small applied magnetic field of 0.1 T. Adding V consistently reduces the compensation temperature from 380 K to 260 K. For y = 0.1, the M-H loop at 300 K in Fig. 1(b) shows a modest increase of the coercivity (< 0.1 T) due to the vanishing net magnetization. The sign reversal of the anomalous Hall effect (AHE) shown in Fig. 2 provides another evidence that the magnetic compensation has indeed achieved near 300 K. In the talk, we will also discuss the effect of V doping on the intrinsic and extrinsic contributions of AHE. 
**References** [1] Joseph Finley and Luqiao Liu, Applied Physics Letters, 116, 110501 (2020)
[2] Se Kwon Kim et al., Nature Materials, 21, 24-34 (2022)
[3] H. Kurt et al., Physical Review Letters, 112, 027201 (2014) 

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Observation of unidirectional spin Hall magnetoresistance in amorphous PtSn4/CoFeB bilayers

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Dependence of TMR and RA on Fe insertion layer thickness in MTJs using L10 (MnCo)Al electrode and MgAl2O4 insulating layer

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