Without manual annotations, unsupervised cross-modal hashing (UCMH) aims to achieve efficient clustering and retrieval by leveraging data interrelationships. However, the retrieval accuracy is constrained by two main aspects: 1) insufficient exploration of data relationships; 2) existing knowledge mining strategies are not well aligned with the architectural properties of multilayer perceptrons. Through summary and error analysis, the human brain is able to achieve fast learning through experience and minimal data. Inspired by this cognitive process, we propose a novel Error Notebook strategy, named ENHash, to more effectively capture similarity information between multi-modal data for fine-grained unsupervised clustering. Firstly, simulating the human process of summarizing experiences, ENHash gradually integrates the information from each batch into a global clustering representation. Secondly, drawing upon human error analysis capabilities, ENHash utilizes the summarized experiences to identify and record incorrectly predicted hash codes. Finally, by leveraging the knowledge derived from this analysis, ENHash guides the hash function to learn fine-grained patterns from the errors. To the best of our knowledge, ENHash represents the first attempt at integrating cognitively-inspired mechanisms into fine-grained UCMH optimization paradigms. We evaluate the proposed ENHash against eight state-of-the-art methods on three widely used datasets and one fine-grained cross-modal dataset. Experimental results show that ENHash achieves substantial improvements over existing approaches. To support reproducibility, the experimental code has been uploaded to the following anonymous repository: https://osf.io/tbehv/?view_only=e4470e710bdf411589391807a2914218.